CLXIX.—The acylation of amides

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Selective α-amination and α-acylation of esters and amides via dual reactivity of O-acylhydroxylamines toward zinc enolates.

Selective α-amination and α-acylation of esters and amides have been developed, employing O-acylhydroxylamines as a dually reactive aminating and acylating reagent. Treatment of zinc enolates with O-acylhydroxylamines provides solely 1,3-dicarbonyl compounds under mild conditions. Introduction of a copper catalyst into the system shifts the reactivity entirely, yielding α-amination products exc...

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ژورنال

عنوان ژورنال: J. Chem. Soc., Trans.

سال: 1904

ISSN: 0368-1645

DOI: 10.1039/ct9048501673